Several high-profile names are now available, including former Real Madrid stars Dani Carvajal and David Alaba, veteran midfielder Dani Parejo, former Spain internationals Marcos Alonso and José Luis Morales, as well as Oscar Mingueza and Cedric Bakambu.
Malaga have the highest number of departing players, with nine members of their squad seeing their contracts expire, while Athletic Club, Atletico Madrid, Barcelona and Real Sociedad had no first-team players out of contract.
Some players are still in talks over new deals or have renewal clauses that could yet be activated, meaning their futures may be resolved in the coming days.
Out-of-contract LaLiga players by club
Osasuna
Juan Cruz
Alaves
Raul Fernandez
Elche
Josan Ferrandez
Getafe
Diego Rico
Domingos Duarte
Allan Nyom
Levante
Pablo Martinez
Diego Pampin
Jose Luis Morales
Mathew Ryan
Malaga
Javi Montero
Eneko Jauregui
Jokin Gabilondo
Einar Galilea
Juanpe
Josue Dorrio
Victor Garcia
Darko Brasanac
Luismi Sanchez
Racing Santander
Jaime Mata
Marco Sangalli
Rayo Vallecano
Abdul Mumin
Luiz Felipe
Alfonso Espino
Celta Vigo
Oscar Mingueza
Marcos Alonso
Franco Cervi
Joseph Aidoo
Mihailo Ristic
Deportivo La Coruna
Sergio Escudero
Ximo Navarro
Cristian Herrera
Espanyol
Fernando Calero
Real Betis
Ricardo Rodriguez
Cedric Bakambu
Real Madrid
David Alaba
Dani Carvajal
Sevilla
Alexis Sanchez
Nemanja Gudelj
Adnan Januzaj
Orjan Nyland
Valencia
Guido Rodriguez
Eray Comert
Thierry Correia
Renzo Saravia
Villarreal
Dani Parejo
Thomas Partey